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Vibrational relaxation and radiative gain in expanding flows of anharmonic oscillators false
By:Robert L. McKenzie,United States. National Aeronautics and Space Administration,Ames Research Center
Published on 1971 by


The set of master rate equations for the vibrational relaxation of mixtures of anharmonic diatomic gases in supersonic nozzle expansions is integrated numerically. Large deviations from a Boltzmann distribution of vibrational state population are predicted, particularly when vibrational energy is exchanged between two near-resonant diatomic species. Radiative gain coefficients for nonequilibrium vibration-rotation transitions are also computed and positive gains, sufficient to support laser oscillations, are predicted for CO-N2 and CO-N,-Ar admixtures.

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